Sagnac-enhanced impulsive stimulated Raman scattering for highly sensitive low-frequency Raman spectroscopy

Femtosecond multiple - pulse impulsive stimulated Raman scattering spectroscopy

Optical control of elementary molecular motion through impulsive stimulated Raman scattering is enhanced by means of timed sequences of femtosecond pulses that are produced by pulse-shaping techniques. In particular, terahertz-rate trains of femtosecond pulses are used for repetitive impulsive excitation of individual phonon modes in an a-perylene molecular crystal. When the pulse repetition ra...

Macroscale Plasmonic Substrates for Highly Sensitive Surface-Enhanced Raman Scattering**

Surface Enhanced Raman Scattering Spectroscopy

This review covers from the basic principles of Raman spectroscopy to the advanced technique of surface enhanced Raman Scattering (SERS) spectroscopy. After briefly going through the description of Raman and introduction of the development of SERS, the article will focus on the “hotspot” of the current research work on SERS – single molecule spectroscopy. We will see later that “hotspot” is als...

Femtosecond time-resolved Raman spectroscopy using stimulated Raman scattering

Femtosecond Raman spectroscopy has been developed to investigate ultrafast photoinduced structural changes of materials. Vibrational modes in the photogenerated transient species are measured by stimulated Raman scattering using a Raman pump pulse with narrow bandwidth and a femtosecond supercontinuum probe pulse. The Raman signal can be measured without slowing the temporal response and broade...

Surface-Enhanced Femtosecond Stimulated Raman Spectroscopy.

Surface-enhanced Raman spectroscopy (SERS) and femtosecond stimulated Raman spectroscopy (FSRS) have revolutionized the Raman spectroscopy field. SERS provides spectroscopic detection of single molecules, and FSRS enables the acquisition of Raman spectra on the ultrafast time scale of molecular motion. Here, we present the first successful combination of these two techniques, demonstrating surf...